- Tytuł:
- Interplay between Correlated Electrons and Quantum Phonons in Charge-Ordered and Mott-Insulating Organic Compounds
- Autorzy:
-
Yonemitsu, K.
Maeshima, N.
Tanaka, Y. - Tematy:
-
78.20.Bh
71.30.+h
71.45.Lr
71.10.Fd - Pokaż więcej
- Wydawca:
- Polska Akademia Nauk. Instytut Fizyki PAN
- Powiązania:
- https://bibliotekanauki.pl/articles/1490009.pdf Link otwiera się w nowym oknie
- Opis:
- At an early stage of the photoinduced transition from an insulator to a metal in quasi-two-dimensional organic conductors, a coherent motion of electrons is observed in a charge-ordered insulator, but not so far in a Mott insulator. The mechanisms of these different photoinduced charge dynamics are theoretically studied by numerical solutions to the time-dependent Schrödinger equation for exact many-electron-phonon wave functions on small clusters of model systems. We use two-dimensional three-quarter-filled extended Holstein-Hubbard models on anisotropic triangular lattices. For a charge-ordered insulator on a lattice simplified from the structure of $α-\text{(BEDT-TTF)}_2I_3$, we indeed find a low-energy collective electronic motion coupled with quantum phonons even if the energy of photoexcitation is away from this energy. For a Mott insulator on a lattice simplified from the structure of $κ-\text{(BEDT-TTF)}_2X$, however, such a collective motion does not appear, and quantum phonons are hardly excited.
- Dostawca treści:
- Biblioteka Nauki
Artykuł